There is another thing you need to do in Rift to make it load balance onto another core.
In the rift.cfg for your characters located in C:\Users\<username>\appdata\local\RIFT (the files are virtualized, so you will see <Charactername>-rift.cfg) look for a setting called Main CPU Thread (it defaulted to 3 on my i7 920). Change that setting to a different core for each account (in my case I set it to maincputhread = 3 on one character and maincputhread = 5 on the other).
If you do that, you will have the primary thread for each account on a different cpu core. After making that change I went from core 3 tapped at 100% to core 3 and 5 tapped at about 80% each.
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